UKCCSRC Call 1 project report: Chemical looping for low-cost oxygen and other applications. Part I (open access)

There were a number of aims of this project - to develop initial flowsheets and designs for CLC with oxygen uncoupling; to model and design reactors; and to produce and test a variety of novel materials for CLC with oxygen uncoupling. The project has succeeded in a number of aims; to develop and test materials (Cambridge), to conduct an initial test of CLC with oxygen uncoupling (the first at scale in the UK, conducted at Cranfield, and the major stated aim of the project - see Figure 2-13), and to model and develop a novel reactor for CLC with oxygen uncoupling (Imperial). Overall, these aspects exceeded the initial project brief. Initial time-dependent flowsheets were developed at Cambridge for CLC processes - unfortunately key staff loss led to a significant hiatus in the activity. Industrial reviewing was limited because of the challenges in developing the flowsheeting activity.